Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+

Investigation in radioactive contaminant removal from aqueous solutions has been considered essential upon unexpected nuclear accidents. In this report, we have successfully prepared Prussian blue analogues (PBAs) with different substituted cations (A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+)). The synthe...

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Những tác giả chính: Lê, Thị Hà Lan, Nguyễn, An Sơn, Nguyễn, Đình Trung, Le, Thi Van Cam, Cao, Hai Van, Nguyen, Ngoc Bao, Le, Thi Thao Phuong
Định dạng: Journal article
Ngôn ngữ:English
Được phát hành: Hindawi 2022
Truy cập trực tuyến:http://scholar.dlu.edu.vn/handle/123456789/1198
https://doi.org/10.1155/2021/5533620
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description Investigation in radioactive contaminant removal from aqueous solutions has been considered essential upon unexpected nuclear accidents. In this report, we have successfully prepared Prussian blue analogues (PBAs) with different substituted cations (A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+)). The synthesized PBAs were characterized and employed for the removal of Cs+, Sr2+, and Co2+ as sorption models, which are commonly found in radioactive waste. Sorption examinations reveal that Cu2[Fe(CN)6] has the highest sorption capacity towards Cs+, Sr2+, and Co2+ compared with those of Co2[Fe(CN)6] and Ni2[Fe(CN)6]. This is mainly attributed to the cation-exchange ability of substituted metal within the framework of PBAs. The sorption mechanism is qualitatively and quantitatively supported by infrared spectroscopy (IR) and total reflection X-ray fluorescence spectroscopy analysis (TXRF). In addition, it was found that Cs+ is adsorbed most effectively by PBAs due to the size matching between Cs+ ions and the channel windows of PBAs. These findings are important for the design of sorbents with suitable ion-exchange capacity and selectivity toward targeted radioactive wastes.
format Journal article
author Lê, Thị Hà Lan
Nguyễn, An Sơn
Nguyễn, Đình Trung
Le, Thi Van Cam
Cao, Hai Van
Nguyen, Ngoc Bao
Le, Thi Thao Phuong
spellingShingle Lê, Thị Hà Lan
Nguyễn, An Sơn
Nguyễn, Đình Trung
Le, Thi Van Cam
Cao, Hai Van
Nguyen, Ngoc Bao
Le, Thi Thao Phuong
Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
author_facet Lê, Thị Hà Lan
Nguyễn, An Sơn
Nguyễn, Đình Trung
Le, Thi Van Cam
Cao, Hai Van
Nguyen, Ngoc Bao
Le, Thi Thao Phuong
author_sort Lê, Thị Hà Lan
title Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
title_short Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
title_full Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
title_fullStr Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
title_full_unstemmed Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+
title_sort prussian blue analogues of a2[fe(cn)6] (a: cu2+, co2+, and ni2+) and their composition-dependent sorption performances towards cs+, sr2+, and co2+
publisher Hindawi
publishDate 2022
url http://scholar.dlu.edu.vn/handle/123456789/1198
https://doi.org/10.1155/2021/5533620
_version_ 1768305964372459520
spelling oai:scholar.dlu.edu.vn:123456789-11982022-10-07T08:37:24Z Prussian Blue Analogues of A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+) and Their Composition-Dependent Sorption Performances towards Cs+, Sr2+, and Co2+ Lê, Thị Hà Lan Nguyễn, An Sơn Nguyễn, Đình Trung Le, Thi Van Cam Cao, Hai Van Nguyen, Ngoc Bao Le, Thi Thao Phuong Investigation in radioactive contaminant removal from aqueous solutions has been considered essential upon unexpected nuclear accidents. In this report, we have successfully prepared Prussian blue analogues (PBAs) with different substituted cations (A2[Fe(CN)6] (A: Cu2+, Co2+, and Ni2+)). The synthesized PBAs were characterized and employed for the removal of Cs+, Sr2+, and Co2+ as sorption models, which are commonly found in radioactive waste. Sorption examinations reveal that Cu2[Fe(CN)6] has the highest sorption capacity towards Cs+, Sr2+, and Co2+ compared with those of Co2[Fe(CN)6] and Ni2[Fe(CN)6]. This is mainly attributed to the cation-exchange ability of substituted metal within the framework of PBAs. The sorption mechanism is qualitatively and quantitatively supported by infrared spectroscopy (IR) and total reflection X-ray fluorescence spectroscopy analysis (TXRF). In addition, it was found that Cs+ is adsorbed most effectively by PBAs due to the size matching between Cs+ ions and the channel windows of PBAs. These findings are important for the design of sorbents with suitable ion-exchange capacity and selectivity toward targeted radioactive wastes. 2021 2022-10-07T08:37:21Z 2022-10-07T08:37:21Z 2021-03-27 Journal article Bài báo đăng trên tạp chí thuộc ISI, bao gồm book chapter http://scholar.dlu.edu.vn/handle/123456789/1198 https://doi.org/10.1155/2021/5533620 en Journal of Nanomaterials 1687-4110 J. 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