Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution

Finding suitable draw solutions is still a major problem when developing FO technologies. This study represents the first time a mixed trivalent draw solution containing of EDTA–2Na and Na3PO4 was systemically studied for FO performance. The objective here was to achieve simultaneously low reverse s...

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Những tác giả chính: Nguyen Cong Nguyen, Duong, Hung Cong, Nguyen Thi Hau, Chen, Shiao-Shing, Le, Huy Quang, Ngo, Huu Hao, Guo, Wenshan, Duong, Chinh Cong, Lê, Ngọc Chung, Bui, Xuan Thanh
Định dạng: Journal article
Ngôn ngữ:English
Được phát hành: 2023
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Truy cập trực tuyến:https://scholar.dlu.edu.vn/handle/123456789/3032
https://www.sciencedirect.com/science/article/pii/S0376738820306086
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spelling oai:scholar.dlu.edu.vn:123456789-30322023-09-28T13:45:28Z Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution Nguyen Cong Nguyen Duong, Hung Cong Nguyen Thi Hau Chen, Shiao-Shing Le, Huy Quang Ngo, Huu Hao Guo, Wenshan Duong, Chinh Cong Lê, Ngọc Chung Bui, Xuan Thanh Forward osmosis; Membrane distillation; Draw solution regeneration; Reverse salt flux; Low-carbon desalination Finding suitable draw solutions is still a major problem when developing FO technologies. This study represents the first time a mixed trivalent draw solution containing of EDTA–2Na and Na3PO4 was systemically studied for FO performance. The objective here was to achieve simultaneously low reverse salt flux and high water flux. The FO results showed that the mixed trivalent draw solution-based 0.3 M EDTA–2Na and 0.55 M Na3PO4 underwent higher water flux (Jw = 9.17 L/m2⋅h) than that of pure 0.85 M EDTA-2Na (Jw = 7.02 L/m2⋅h) due to its lower viscosity. Additionally, the specific reverse salt flux caused by mixing 0.3 M EDTA–2Na with 0.55 M Na3PO4 draw solution was only 0.053 g/L using DI water as the feed solution. Donnan equilibrium force and formed complexation of [EDTANa]3-, [HPO4Na]- with the FO membrane are believed to constitute the main mechanism for minimizing salt leakage from the mixed draw solution. Moreover, the FO desalination process utilizing the mixed trivalent draw solution achieved water fluxes of 6.12 L/m2⋅h with brackish water (TDS = 5000 mg/L) and 3.10 L/m2⋅h with seawater (TDS = 35,000 mg/L) as the feed solution. Lastly, diluted mixed trivalent draw solution following the FO process was effectively separated using the MD process with salt rejection >99.99% at a mild feed temperature of 55 °C. 2023-09-28T13:45:23Z 2023-09-28T13:45:23Z 2020-05-15 Journal article Bài báo đăng trên tạp chí thuộc ISI, bao gồm book chapter 0376-7388 https://scholar.dlu.edu.vn/handle/123456789/3032 10.1016/j.memsci.2020.118029 https://www.sciencedirect.com/science/article/pii/S0376738820306086 en
institution Thư viện Trường Đại học Đà Lạt
collection Thư viện số
language English
topic Forward osmosis; Membrane distillation; Draw solution regeneration; Reverse salt flux; Low-carbon desalination
spellingShingle Forward osmosis; Membrane distillation; Draw solution regeneration; Reverse salt flux; Low-carbon desalination
Nguyen Cong Nguyen
Duong, Hung Cong
Nguyen Thi Hau
Chen, Shiao-Shing
Le, Huy Quang
Ngo, Huu Hao
Guo, Wenshan
Duong, Chinh Cong
Lê, Ngọc Chung
Bui, Xuan Thanh
Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
description Finding suitable draw solutions is still a major problem when developing FO technologies. This study represents the first time a mixed trivalent draw solution containing of EDTA–2Na and Na3PO4 was systemically studied for FO performance. The objective here was to achieve simultaneously low reverse salt flux and high water flux. The FO results showed that the mixed trivalent draw solution-based 0.3 M EDTA–2Na and 0.55 M Na3PO4 underwent higher water flux (Jw = 9.17 L/m2⋅h) than that of pure 0.85 M EDTA-2Na (Jw = 7.02 L/m2⋅h) due to its lower viscosity. Additionally, the specific reverse salt flux caused by mixing 0.3 M EDTA–2Na with 0.55 M Na3PO4 draw solution was only 0.053 g/L using DI water as the feed solution. Donnan equilibrium force and formed complexation of [EDTANa]3-, [HPO4Na]- with the FO membrane are believed to constitute the main mechanism for minimizing salt leakage from the mixed draw solution. Moreover, the FO desalination process utilizing the mixed trivalent draw solution achieved water fluxes of 6.12 L/m2⋅h with brackish water (TDS = 5000 mg/L) and 3.10 L/m2⋅h with seawater (TDS = 35,000 mg/L) as the feed solution. Lastly, diluted mixed trivalent draw solution following the FO process was effectively separated using the MD process with salt rejection >99.99% at a mild feed temperature of 55 °C.
format Journal article
author Nguyen Cong Nguyen
Duong, Hung Cong
Nguyen Thi Hau
Chen, Shiao-Shing
Le, Huy Quang
Ngo, Huu Hao
Guo, Wenshan
Duong, Chinh Cong
Lê, Ngọc Chung
Bui, Xuan Thanh
author_facet Nguyen Cong Nguyen
Duong, Hung Cong
Nguyen Thi Hau
Chen, Shiao-Shing
Le, Huy Quang
Ngo, Huu Hao
Guo, Wenshan
Duong, Chinh Cong
Lê, Ngọc Chung
Bui, Xuan Thanh
author_sort Nguyen Cong Nguyen
title Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
title_short Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
title_full Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
title_fullStr Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
title_full_unstemmed Forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
title_sort forward osmosis–membrane distillation hybrid system for desalination using mixed trivalent draw solution
publishDate 2023
url https://scholar.dlu.edu.vn/handle/123456789/3032
https://www.sciencedirect.com/science/article/pii/S0376738820306086
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