Dipolar Correlation Spectroscopy (Higher-Order Correlation Terms in Three-Spin Double Electron Electron Resonance (DEER))
This master thesis presents experimental conditions which allow to ex tract the three-spin contribution precisely from experimental DEER signals. Broadband chirp pulses, generated by a fast arbitrary waveform generator (AWG), were used as DEER pump pulses in combination with a homebuilt, highly...
Đã lưu trong:
| Tác giả chính: | |
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| Định dạng: | Sách |
| Ngôn ngữ: | English |
| Được phát hành: |
Springer
2015
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| Những chủ đề: | |
| Truy cập trực tuyến: | https://scholar.dlu.edu.vn/thuvienso/handle/DLU123456789/56235 |
| Các nhãn: |
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| Thư viện lưu trữ: | Thư viện Trường Đại học Đà Lạt |
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| Tóm tắt: | This master thesis presents experimental conditions which allow to ex
tract the three-spin contribution precisely from experimental DEER signals.
Broadband chirp pulses, generated by a fast arbitrary waveform generator
(AWG), were used as DEER pump pulses in combination with a homebuilt,
highly overcoupled microwave resonator. This experimental setup was tested
on triply labeled nitroxide radicals and a Gd(III)-nitroxide radical. To
evaluate the quality of the extracted two-spin and three-spin contribution,
simulations were performed.... |
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