XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay
This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is s...
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2016
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oai:scholar.dlu.edu.vn:DLU123456789-597262023-11-11T06:48:14Z XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay Schnorr, Kirsten Diatomic molecules Electrochemical analysis This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy. 2016-03-01T07:15:34Z 2016-03-01T07:15:34Z 2015 Book 978-3-319-12139-0 978-3-319-12138-3 https://scholar.dlu.edu.vn/thuvienso/handle/DLU123456789/59726 en application/pdf Springer |
| institution |
Thư viện Trường Đại học Đà Lạt |
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Thư viện số |
| language |
English |
| topic |
Diatomic molecules Electrochemical analysis |
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Diatomic molecules Electrochemical analysis Schnorr, Kirsten XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| description |
This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy. |
| format |
Book |
| author |
Schnorr, Kirsten |
| author_facet |
Schnorr, Kirsten |
| author_sort |
Schnorr, Kirsten |
| title |
XUV Pump-Probe Experiments on Diatomic Molecules:
Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| title_short |
XUV Pump-Probe Experiments on Diatomic Molecules:
Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| title_full |
XUV Pump-Probe Experiments on Diatomic Molecules:
Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| title_fullStr |
XUV Pump-Probe Experiments on Diatomic Molecules:
Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| title_full_unstemmed |
XUV Pump-Probe Experiments on Diatomic Molecules:
Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay |
| title_sort |
xuv pump-probe experiments on diatomic molecules:
tracing the dynamics of electron rearrangement and interatomic coulombic decay |
| publisher |
Springer |
| publishDate |
2016 |
| url |
https://scholar.dlu.edu.vn/thuvienso/handle/DLU123456789/59726 |
| _version_ |
1782550089059794944 |